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Because of the increasing need for renewable sources of energy, substantial effort is dedicated to the development of novel types of solar cells Siliconbased cells have reached large-scale production and can be operated under varying environmental conditions However, costly and elaborate production technology has spurred the search for alternative concepts beyond the siliconbased technology In particular, it would be desirable to substitute costly semiconductors by cheap and abundant compounds, such as metal oxide lms, which can be obtained by evaporation-induced self-assembly in combination with sol-gel chemistry or the deposition of mesoporous powder (eg, by doctor-blading) Dye-sensitized solar cells (DSSCs) have already been shown to allow for promising light-to-electricity conversion ef ciencies of up to 10% for certain types.

Error Probability for Coherent Receivers Antipodal Signaling For antipodal signals, the pairwise error probability is: Prpair (sj , sk ) = Q S (1 Re{ j k }) (12.30) (12.31)

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Figure 3.3.18 (a) Principal arrangement of the position-sensitive X-ray spectrometer. (b) Spectral separation in a Tispectrum by means of the system in (a)

44 The classic Graetzel -type cell uses TiO2 as an n-type semiconductor and a suitable dye and electrolyte, but also other metal oxides are discussed to serve as the charge carrier81 In general, the oxide has to be in a highly crystalline state in order to ful ll the requirements for a semiconductor with suf cient conductivity and chemical stability In short, the classic Graetzel-type DSSC works as follows (see the review of L M Peter81 for an overview): Photocurrents in the DSSC are created when light is absorbed by the sensitizer dye, leading to electron injection into the conduction band of TiO2 The electrons move through the TiO2 network by a random walk process until they reach the electrode The dye is regenerated by electron transfer from iodide before it has time to undergo bleaching.

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591 1045 614

The I3- ions produced in the regeneration step diffuse to the cathode (usually covered with platinum), where they are reduced to iodide ions completing the regenerative cycle Alternative concepts use mesoporous TiO2 in combination with conducting polymers Up until some years ago, the TiO2 used in DSSCs was mainly of coarse-grain morphology, ie, with particle sizes on the scale of >100 nm Although the performance of DSSCs is regarded as being dependent on various parameters (eg, electrolyte and dye), it is generally assumed that modi cation of the semiconductor morphology still has the potential to lead to a signi cant enhancement of the ef ciency.

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